Iceland is about 1.8 times bigger than Croatia.

Croatia is approximately 56,594 sq km, while Iceland is approximately 103,000 sq km, making Iceland 82% larger than Croatia. Meanwhile, the population of Croatia is ~4.2 million people (3.8 million fewer people live in Iceland).
This to-scale comparison of Croatia vs. Iceland uses the Mercator projection, which distorts the size of regions near the poles. Learn more.

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